
Research
Interest:
Research
interest lies at the interface of biology and the physical sciences. The
general thrust
of
my research program is aimed at developing and applying computational
methodologies to
understand
structural characteristics, kinetics and thermodynamics of peptides, proteins
and
carbohydrates.
Research
Capabilities:
Molecular
Dynamics Simulations
Enhanced
sampling methods
Molecular
Modeling & Forcefields
Coarse-grained
approaches
Free
energy and binding calculations
Research
Programs:
Our basic
science research program is aligned towards supporting emerging national
security
missions.
We apply our expertise in computational structural biology/immunology
capabilities
towards
both health and energy securities.
Research
Projects:
* Dynamics
of surface proteins of HIV & Rational vaccine design
* Protein
Folding & Secondary structural propensities of peptides
*
Aggregation and misfolding of disease related peptides
* Protein
conformational networks and folding pathways
*
Interfacing All-atom simulations with spectral measurements
*
Perturbation of local solvent and protein structures by metals
*
Multi-scale Modeling of Plant Cell Wall Components
*
Pretreatment and Enzymatic degradation of cellulose
* Rational
enzyme design: Increasing turnover and Biasing chirality
Publications:
S. Gnanakaran, B. Scott,
T.M McCleskey and A. E. Garcia. Perturbation of Local Solvent Structure
by a Small Dication:
Structural, Spectroscopic and
Reactive Properties of Beryllium Ion in Water, J. Phys. Chem. B, in press.
Erzsebet
Ravasz, S. Gnanakaran, Zoltan Toroczkai, Network Structure of Protein Folding
Pathways, submitted.
Brian L.
Scott, T. Mark McCleskey, Anu Chaudhary, Elizabeth Hong-Geller, and S.
Gnanakaran, The bioinorganic chemistry
and
associated immunology of Chronic Beryllium Disease, Chem. Comm., accepted.
S. Gnanakaran, Dorothy Lang, Marcus
Daniels, Tanmoy Bhattacharya, Cynthia A. Derdeyn, and Bette Korber. 2007. Clade
Specific Differences in HIV-1: Diversity and Correlations in C3-V4 Regions of
gp120. J. Virol.
81:4886-4891.
Rong, R.,
S. Gnanakaran, J.M. Decker, F. Bibollet-Ruche, J. Taylor, J.N. Sfakianos, J.L.
Mokili, M. Muldoon, J. Mulenga, S. Allen, B.H. Hahn, G.M. Shaw, J.L. Blackwell,
B.T. Korber, E. Hunter, and C.A. Derdeyn. 2007. Unique Mutational patterns in
the envelope 2 amphipathic helix and acquisition of length in gp120
hypervariable domains are associated with resistance to autologous
neutralization of subtype C HIV type 1. J. Virol. 81:5658-5668.
M.
Vuyisich, S. Gnanakaran, J.A. Lovchik, CR. Lyons, K.L. DeBord, and G. Gupta.
2007. Novel therapy for anthrax. J. Biomol. Struct. Dyn. 24:727-728.
S.
Gnanakaran, R. Nussinov, and A.E. Garcia. 2006. Atomic level description of
amyloid beta dimer formation. J. Am. Chem. Soc. 128:2158-2159.
W. Blay, S.
Gnanakaran, B. Foley, N. Doria-Rose, B.T. Korber, and N.L. Haigwood. 2006. Consistent
Patterns of Change During Divergence of Human Immunodeficiency Virus Type 1
Envelope in SHIV-Infected Macaques. J. Virol. 80:999-1014.
S.
Gnanakaran and A.E. Garcia. 2005. Helix-coil transition of alanine peptides in
water: Force field dependence on the folded and unfolded structures. Proteins-Structure
Function and Genetics. 59:773-782.
D. Paschek,
S. Gnanakaran, and A.E. Garcia. 2005. Simulations of the pressure and
temperature unfolding of an alpha-helical peptide. Proc. Natl. Acad. Sci.
USA. 102:6765-6770.
S.
Gnanakaran, R.M. Hochstrasser, and A.E. Garcia. 2004. Nature of structural
inhomogeneities on folding a helix and their influence on spectral
measurements. Proc. Natl. Acad. Sci. USA. 101:9229-9234.
H. Nymeyer,
S. Gnanakaran, and A.E. Garcia. 2004. Atomic simulations of protein folding,
using the replica exchange algorithm. Methods Enzymol. 383:119-149.
S. Gnanakaran and A.E. Garcia. 2003.
Validation of an all-atom protein force field: From dipeptides to larger
peptides. J. Phys. Chem. B. 107:12555-12557.
S. Gnanakaran, H. Nymeyer, J.
Portman, K. Sanbonmatsu, and A.E. Garcia. 2003. Peptide folding simulations.
Curr. Opin. Struct. Biol. 13:168-174.
S. Gnanakaran and A.E. Garcia. 2003.
Folding of a highly conserved diverging turn motif from the SH3 domain. Biophys.
J. 84:1548-1562.
R.M. Hochstrasser, N. Ge, S.
Gnanakaran, and M. Zanni. 2002. Two dimensional infrared spectroscopy: Studies
of the dynamics of structures with femtosecond pulse Fourier transform
correlation spectroscopy. Bull. Chem. Soc. Japan. 75:1103.
S. Gnanakaran and R.M. Hochstrasser.
2001. Conformational preferences of short peptides in relation to
multidimensional IR spectroscopy. J. Am. Chem. Soc. 123:12886-12898.
M.T. Zanni, S. Gnanakaran, J.
Stenger, and R.M. Hochstrasser. 2001. Two-dimensional infrared spectroscopy of
solvent dependent conformations of acetylproline-NH2. J. Phys. Chem. 105:6520-6535.
S. Gnanakaran, G. Haran, R. Kumble,
and R.M. Hochstrasser. 1999. Energy transfer and localization: Applications to
photosynthetic systems. Chapter in book titled ÒResonance Energy TransferÓ. J. Wiley Publishing Co.
S. Gnanakaran and R.M. Hochstrasser.
1999. Effect of vibrational coherence on rotational dynamics in solution. Int.
J. Quantum Chem.
72:451-462.
S. Gnanakaran, M. Lim, M. Volk, E.
Gooding, Y. Kholodenko, and R.M. Hochstrasser. 1998. Chemical reaction dynamics
of some simple molecules in solution. Phil. Trans. R. Soc. Lond. A. 356:377-388.
M. Volk, S. Gnanakaran, M. Lim, E.
Gooding, Y. Kholodenko, and R.M. Hochstrasser. 1997. Anisotropy measurements of
the solvated HgI2; Transition state and fragment rotational dynamics. J.
Phys. Chem. A.101:638-643.
M. Lim, S. Gnanakaran, and R.M.
Hochstrasser. 1997. Charge shifting in the ultrafast photo-reactions of ClO-
in water. J. Chem. Phys. 106:3485-3493.
S. Gnanakaran and R.M. Hochstrasser.
1996. Vibrational relaxation of HgI in ethanol: Equilibrium molecular dynamics
simulations. J. Chem. Phys. 105:3486-3496.
N. Pugliano, S. Gnanakaran, and R.M.
Hochstrasser. 1996. The dynamics of photo-dissociation reaction. J.
Photochem. & Photobiol. A. 102:21-28.
N. Pugliano, A. Szarka, S.
Gnanakaran, and R.M. Hochstrasser. 1995. Vibrational populational dynamics of
the HgI photofragment in ethanol solution. J. Chem. Phys. 103:6498-6511.
K. Wynne, S. Gnanakaran, C. Galli,
F. Zhu, and R.M. Hochstrasser. 1994. Luminescence studies of ultrafast energy transfer
oscillations in dimmers. J. Lumin. 60-1:735-738.
P.G. Smith, S. Gnanakaran, A.G.
Kasziska, A.L. Motyka, S.M. Hong, R.M. Hochstrasser, and M. Topp. 1994.
Electronic coupling and conformational barrier crossing of 9Õ,9-Bifluorenyl
studied in a supersonic jet. J. Chem. Phys. 100:3384-3493.